What's the best way to move c:\users to d:\users under vista/Window 7

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The easiest and recommended way is to move the individual special folders inside a user directory, such as Documents, Music, Video’s, etc. You can do this with the following steps:
Right click –> properties
Location tab Fill in the desired location and
click ‘move’
Downside to this is that this still leaves the main ‘Users’ folder inplace.